The objective of this research was to examine the mechanisms of FeCO 3, Na 2 CO 3, and FeCO 3Na 2 CO 3 based catalytic coal gasification of a lowsulfur subbituminous Wyodak coal from the Powder River Basin (PRB) of Wyoming. Xray diffraction (XRD), Mössbauer spectroscopy, scanning electron microscopy (SEM), Fourier transform infrared spectroscopy (FTIR), gas chromatography (GCMS) and ...
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Popa et al. [13]. studied the catalytic steam gasification of a Powder River Basin coal using Na 2 CO 3, and the results demonstrated that the total amounts of H 2, CO, CO 2 and CH 4 generated during the entire gasification with 5 g of dry ashfree coal were,, and mol, respectively, while correspondingly, those with catalyst ...
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Competition and Inhibition Effects during Coal Char Gasification in the Mixture of H2O and CO2. Rui Zhang, Q. H. Wang, Zhongyang Luo, M. Fang, K. Cen. Chemistry. 2013. The mechanisms of char gasification in the mixture of H2O and CO2 are not clear, and some problems are yet to be solved. The LangmuirHinshelwood (LH) model of char ...
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CO 2 gasification of Wyodak lowsulfur subbituminous coal from the Powder River Basin (PRB) of Wyoming was conducted in a fixedbed laboratory gasifier at atmospheric pressure with Na 2 CO 3, an inexpensive catalyst widely available in Wyoming. The sodium effect on the coal pyrolysis and the sodium forms existing during the char gasification were investigated using thermogravimetric ...
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The gasification experiments of coal chars with CO2 were carried out isothermally, with K, Ca, Ni, and Zn chloride catalysts, adopting a thermal gravimetric analyzer (TGA) from 800 to 1100 °C. The kinetic characteristic of the samples were described using the volumetric model (VM), the grain model (GM), and the random pore model (PRM). The morphology patterns of the samples were tested ...
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The catalytic mechanism is generally described as the added metal element contacting with gasifying agent (H 2 O and/or CO 2 ) produces hydrogen and/or carbon monoxide and a layer of...
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CO2 gasification of Powder River Basin coal catalyzed by a costeffective and environmentally friendly iron catalyst journal, May 2015. Zhang, Fan; Xu, Deping; Wang, Yonggang; ... (GPE) concept for producing synthetic natural gas and hydrogen from coal involves the catalytic gasification of coal and carbon. GPE's technology "refines" coal ...
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Variation of Char Reactivity during Catalytic Gasification with Steam: Comparison among Catalytic Gasification by IonExchangeable Na, Ca, and Na/Ca Mixture. ... Characterization of Powder River Basin coal pyrolysis with costeffective and environmentallyfriendly composite Na Fe catalysts in a thermogravimetric analyzer and a fixedbed reactor.
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In this study, DFT is used to search for possible CO2 gasification paths at the two char edges (armchair edge and zigzag edge) catalyzed by Fe. The optimal reaction path is determined by path ...
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CO2 gasification of Powder River Basin coal catalyzed by a costeffective and environmentally friendly iron catalyst. Full Record; Other Related Research; Authors: Zhang, Fan; Xu, Deping; Wang, Yonggang; Argyle, Morris D.; Fan, Maohong Publication Date: Fri May 01 00:00:00 EDT 2015 Sponsoring Org.: USDOE
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As a result, fuels with larger surface area and more catalytic components in ash were preferred for increasing the intrinsic reactivity of CO2 gasification particularly for lowrank coals and biomass, respectively. ... Reaction kinetics of Powder River Basin coal gasification in carbon dioxide using a modified drop tube reactor, Fuel, 140 (2015 ...
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CO capture and utilization caused more and more public attention because of its environmental impact. The objective of this work was to study the catalytic gasification of a subbituminous coal from the Powder River Basin (PRB) using a CO and HO mixture as the gasifying agent. Sodium and iron, in the form of inexpensive compounds, were chosen to catalyze the coal gasification. The experiments ...
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CO2 capture and utilization caused more and more public attention because of its environmental impact. The objective of this work was to study the catalytic gasification of a subbituminous coal from the Powder River Basin (PRB) using a CO2 and H2O mixture as the gasifying agent. Sodium and iron, in the form of inexpensive compounds, were chosen to catalyze the ...
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Popa et al. [13]. studied the catalytic steam gasification of a Powder River Basin coal using Na2CO3, and the results demonstrated that the total amounts of H2, CO, CO2 and CH4 generated during the entire gasification with 5 g of dry ashfree coal were,, and mol, respectively, while correspondingly, those with catalyst were ...
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Highquality oil and gas from pyrolysis of Powder River Basin coal catalyzed by an environmentallyfriendly, inexpensive composite ironsodium catalysts Article Dec 2017
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A study was carried out in both inert and CO 2 atmosphere to investigate the interaction mechanism of K 2 CO 3 with graphite and coal char during the catalytic gasification of coal char. The formation of K 2 CO 3 catalytic precursors was identified by using series of different techniques. The results obtained in an inert atmosphere show that the interaction between K 2 CO 3 and carbon readily ...
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DOI: / Corpus ID: ; Catalytic gasification of a Powder River Basin coal article{Popa2013CatalyticGO, title={Catalytic gasification of a Powder River Basin coal}, author={T. Popa and Maohong Fan and Morris D. Argyle and Rachid B. Slimane and David A. Bell and Brian Towler}, journal={Fuel}, year={2013}, volume={103}, pages={161170}, url={https://api ...
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The objective of this work was to study the catalytic gasification of a subbituminous coal from the Powder River Basin (PRB) using a CO2 and H 2O mixture as the gasifying agent. Sodium and iron, in the form of inexpensive compounds, were chosen to catalyze the coal gasification.
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Most of the coal produced in the PRB supports electric power generation in the United States. Starting in the 1990s, many coalfired power plants switched to subbituminous coal from the PRB—which has relatively low sulfur content—to meet tightening Clean Air Act emission 2003, the Powder River Basin yielded more coal than the Appalachian coal basins in the eastern United States.
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Catalytic gasification of a Wyodak lowsulfur subbituminous coal from the Powder River Basin of Wyoming was investigated using an inexpensive catalyst, Na 2 CO 3, widely available in Wyoming. Experiments were performed in an atmospheric pressure fixedbed laboratory gasifier.
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Semantic Scholar extracted view of "Gasification of a South Australian lowrank coal with carbon dioxide and steam: kinetics and reactivity studies" by D. Ye et al. ... Catalytic gasification of a Powder River Basin coal with CO2 and H2O mixtures. ... This work reports on a kinetic study on the gasification of Brazilian mineral coal with steam ...
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Due to the serious impact of accelerating global climate change, the United States and China signed the China Joint Announcement on Climate Change in 2014, which imposed significant restrictions on the coal industry.
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CO 2 gasification of Wyodak lowsulfur subbituminous coal from the Powder River Basin (PRB) of Wyoming was conducted in a fixedbed laboratory gasifier at atmospheric pressure with Na 2 CO 3, an inexpensive catalyst widely available in sodium effect on the coal pyrolysis and the sodium forms existing during the char gasification were investigated using thermogravimetric analyses ...
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Abstract. Catalytic gasification of a Wyodak lowsulfur subbituminous coal from the Powder River Basin of Wyoming was investigated using an inexpensive catalyst, Na2CO3, widely available in ...
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DOI: / Corpus ID: ; Characterization of the mechanism of gasification of a powder river basin coal with a composite catalyst for producing desired syngases and liquids
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The YN coal samples were manually ground and sieved to particle sizes mm. The pyrolysis of coal samples and char gasification was carried out in a fixed bed reactor. The experimental setup is shown in Fig. 1. The quartz tube used in this work has an inner diameter of 5 cm and length of 22 cm, the
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Gasification of biomass with CO 2 and H 2 O mixtures in a catalytic fluidised bed. Fuel 2017, 210, 605610. DOI: / Ying Wang, David A. Bell. Competition between H 2 O and CO 2 during the gasification of Powder River Basin coal. Fuel 2017, 187, 94102. DOI: /
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As the largest coal mining region and the main coal supply in the United States, Powder River Basin (PRB) coal has a tight connection with this country's power industry and requires special attention in coal gasification studies. Very little investigation of PRB gasification rates in the presence of both CO 2 and steam have been done. As a ...
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This kinetics arose from noncatalytic gasification. AAEM species remaining in the char had no catalytic activity. ... Catalytic gasification of a Powder River Basin coal with CO2 and H2O mixtures. Fuel Processing Technology 2017, 161, ... Analysis of Catalytic Gasification with Calcium in Coal Gasification Process by Extended Random Pore Model.
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The objective of this work was to study the catalytic gasification of a subbituminous coal from the Powder River Basin (PRB) using a CO 2 and H 2 O mixture as the gasifying agent. Sodium and iron, in the form of inexpensive compounds, were chosen to catalyze the coal gasification.
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